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Polymerization of methylmethacrylate by tridentate schiff base berivative of indenyl and cyclooctatetraenyl lanthanoid complexes along with Al(i-Bu)/sub 3/ catalytic system

Abstract

Different types of the tridentate Schiff base, [N-(2-methoxyphenyl) salicylideneamine] derivative of lanthanoid complexes along with Al(i-Bu)/sub 3/ are proved to be versatile tools for the polymerization of methylmethacrylate (MMA). The complexes, derived from indene and tridentate Schiff base ligands, express better efficiency (Mv = 195 X 10/sup 3/ - 355 X 10/sup 3/) than the complexes, prepared from cyclooctatetraene (COT) and tridentate Schiff base ligands (Mv=105 X 10/sup 3/ - 175 X 10/sup 3/). The effect of catalyst, temperature, catalyst/MMA molar ratio and catalyst/Al(i-Bu)/sub 3/ molar ratio on the polymerization of MMA at 70 deg. C are studied. It is observed that ligand size and radius of the metal are important factors in determining the catalytic efficiency of the complexes.
Authors:
Yousaf, M; Ali, K G; Chahta, S A.S.; [1]  Ahmad, H B; [2]  Khan, K M [3] 
  1. Government College University, Faisalabad-38040 (Pakistan). Department of Chemistry
  2. Bahauddin Zakariya University, Multan-60800 (Pakistan). Department of Chemistry
  3. University of Karachi (Pakistan). HEJ Research Institute of Chemistry, International Centre for Chemical and Biological Sciences
Publication Date:
Apr 15, 2011
Product Type:
Journal Article
Resource Relation:
Journal Name: Journal of the Chemical Society of Pakistan; Journal Volume: 33; Journal Issue: 2
Subject:
37 INORGANIC, ORGANIC, PHYSICAL AND ANALYTICAL CHEMISTRY; LANTHANUM COMPLEXES; LIGANDS; METHACRYLIC ACID ESTERS; POLYMERIZATION; SCHIFF BASES; CARBOXYLIC ACID ESTERS; CHEMICAL REACTIONS; COMPLEXES; ESTERS; IMINES; ORGANIC COMPOUNDS; ORGANIC NITROGEN COMPOUNDS; RARE EARTH COMPLEXES
OSTI ID:
21493958
Country of Origin:
Pakistan
Language:
English
Other Identifying Numbers:
Journal ID: ISSN 0253-5106; TRN: PK1100502085690
Submitting Site:
INIS
Size:
page(s) 255-259
Announcement Date:
Nov 07, 2011

Citation Formats

Yousaf, M, Ali, K G, Chahta, S A.S., Ahmad, H B, and Khan, K M. Polymerization of methylmethacrylate by tridentate schiff base berivative of indenyl and cyclooctatetraenyl lanthanoid complexes along with Al(i-Bu)/sub 3/ catalytic system. Pakistan: N. p., 2011. Web.
Yousaf, M, Ali, K G, Chahta, S A.S., Ahmad, H B, & Khan, K M. Polymerization of methylmethacrylate by tridentate schiff base berivative of indenyl and cyclooctatetraenyl lanthanoid complexes along with Al(i-Bu)/sub 3/ catalytic system. Pakistan.
Yousaf, M, Ali, K G, Chahta, S A.S., Ahmad, H B, and Khan, K M. 2011. "Polymerization of methylmethacrylate by tridentate schiff base berivative of indenyl and cyclooctatetraenyl lanthanoid complexes along with Al(i-Bu)/sub 3/ catalytic system." Pakistan.
@misc{etde_21493958,
title = {Polymerization of methylmethacrylate by tridentate schiff base berivative of indenyl and cyclooctatetraenyl lanthanoid complexes along with Al(i-Bu)/sub 3/ catalytic system}
author = {Yousaf, M, Ali, K G, Chahta, S A.S., Ahmad, H B, and Khan, K M}
abstractNote = {Different types of the tridentate Schiff base, [N-(2-methoxyphenyl) salicylideneamine] derivative of lanthanoid complexes along with Al(i-Bu)/sub 3/ are proved to be versatile tools for the polymerization of methylmethacrylate (MMA). The complexes, derived from indene and tridentate Schiff base ligands, express better efficiency (Mv = 195 X 10/sup 3/ - 355 X 10/sup 3/) than the complexes, prepared from cyclooctatetraene (COT) and tridentate Schiff base ligands (Mv=105 X 10/sup 3/ - 175 X 10/sup 3/). The effect of catalyst, temperature, catalyst/MMA molar ratio and catalyst/Al(i-Bu)/sub 3/ molar ratio on the polymerization of MMA at 70 deg. C are studied. It is observed that ligand size and radius of the metal are important factors in determining the catalytic efficiency of the complexes.}
journal = {Journal of the Chemical Society of Pakistan}
issue = {2}
volume = {33}
place = {Pakistan}
year = {2011}
month = {Apr}
}